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-ray spectroscopic methodsFurutaka, Kazuyoshi
JNC TN8400 2000-028, 70 Pages, 2000/10
JNC-TN8400-2000-028.pdf:1.71MB
This report describes the study done by the author as a postdoctoral research associate at Japan Nuclear Cycle Development Institute. This report is divided into two parts: improvements in accuracy in determination of thermal neutron capture cross sections, and improvements in accuracy of photo-nuclear absorption cross section measurements using the HHS. (1)In the measurements of thermal neutron capture cross sections using an activation method, accuracies of the final results attained are limited by (1) accuracy of -ray peak detection efficiencies, and (2) accuracies of -ray emission probabilities. In this study; to determine thermal neutron capture cross sections more accurately, the following researches have been done using a newly developed three-dimensional coincidence measurement system: (1)accurate determination of -ray standard sources using a - coincidence method, for precise calibration of -ray peak detection efficiency, and (2) development of a 
- coincidence measurement system using a plastic scintillation detector as a -ray detector, for the determination of -ray emission probabilities of short-lived nuclides, and measurement of -ray emission probabilities of 
Tc nuclide using the coincidence system. (2)To transform radioactive nuclides with small thermal neutron capture cross sections, use of photonuclear absorption reaction has been suggested. In order to transform these nuclides efficiently using the reaction, one has to know detailed behavior of the photo-absorption cross sections. In this study, a Monte-Carlo simulation code has been used to create a standard set of -ray response functions of the high-resolution high-energy spectrometer (HHS), to enable reliable analyses of the data obtained by the spectrometer.
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JNC TJ9400 2000-009, 63 Pages, 2000/02
JNC-TJ9400-2000-009.pdf:2.48MB
The present status of nuclear data for technetium (Tc)-99, which is a well-known fission product (FP), has been reviewed and investigated. And making use of the Kyoto university Lead Slowing-down Spectrometer (KULS), the cross section of the 
Tc (n, ) Tc reaction has been measured in the energy range from thermal to keV neutron energy with an Ar-gas proportinal counter. The neutron flux/spectrum has been monitored with a BF
proportional counter, and the relative measurement has been normalized to the well-known standard capture cross section value for the Tc (n, ) Tc reaction at 0.0253 eV. Self-shielding corrections, especially near the resonance peaks, were made by the calculations with the MCNP code. Although the experimental data measured by Chou et al with a lead slowing-down spectrometer are higher in general, the energy dependency is similar to the present measurement. The evaluated data in ENDF/B-VI and JENDL-3.2 are higher near the resonances at 5.6 and 20 eV and above several 100 eV. A lead slowing-down spectrometer was installed coupled to a 46 MeV electron linac at the Research Reactor Institute, Kyoto university (KURRI). Characteristics of the Kyoto University Lead Slowing-down Spectrometer (KULS) were measured and (1)the relation between neutron slowing-down time t(
s) and energy E(keV) (E=190/t
in Bi hole and E=156/t in Pb hole) and (2)the energy resolution (
40% in Bi and Pb holes) were experimentally investigated. (3)The neutron energy spectrum in the KULS was also measured by the neutron TOF method. The results obtained by the MCNP code were in general agreement with these experimental ones.
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JNC TJ9400 2000-008, 61 Pages, 2000/02
For studies on nuclear transmutation of long-lived fission products (LLFPs) in a fast reactor, detailed characteristics of reactor core such as transmutation performance have to be investigated, so accurate neutron cross section data of LLFPs become necessary. Therefore, the keV-neutron capture cross sections of Tc-99, which is one of important LLFPs, were measured in the present study to obtain the accurate data. The measurement was relative to the standard capture cross sections of Au-197. A neutron time-of-flight method was adopted with a ns-pulsed neutron source by a Pelletron accelerator and a large anti-Compton NaI(TI) gamma-ray detector. As a result, the capture cross sections of Tc-99 were obtained with the error of about 5 % in the incident neutlon energy region of 10 to 600 keV. The present data were compared with other experimental data and the evaluated values of JENDL-3.2, and it was found that the evaluations of JENDL-3.2 were 15-20 % smaller than the present measurements.